Member of Yale faculty since 1977.
Not accepting lab members at this time.
Research Interests
- Inorganic Chemistry
- Organic Chemistry
- Organometallic
- Research
Member of Yale faculty since 1977.
Not accepting lab members at this time.
Carole Velleca
carole.velleca@yale.edu
CRB 230
Design and synthesis of inorganic, coordination and organometallic molecules with unusual structures and properties. These are typically catalytic and electrocatalytic properties for atom economic (green) transformations, bioinorganic relevance or utility in alternative energy strategies, such as solar energy, nitrogen fixation, ammonia oxidation and hydrogen storage.
B.A. New College, Oxford 1970
Ph.D. Sussex University 1973
Postdoctoral Fellow, CNRS, Gif-s-Yvette, France, 1973-75
Attaché de Recherche, Gif, 1975-77
Liu, H-Y.; Lant, H.; Troiano, J.; Hu, G.; Mercado, B.; Crabtree, R. H.; Brudvig, G. W. Electrocatalytic, Homogeneous Ammonia Oxidation in Water to Nitrate and Nitrite with a Copper Complex. J. Am. Chem. Soc. 2022, 144, 8449-8453.
Crabtree, R. H. Alternate Strategies for Solar Fuels from Carbon Dioxide. ACS Energy Lett. 2020, 5, 2505-2507. DOI: 10.1021/acsenergylett.0c01359
Weber, J.; Hasanayn, F.; Fataftah, M.; Mercado, B.Q.; Crabtree, R. H.; Holland, P., Electronic and Spin-State Effects on Dinitrogen Splitting to Nitrides in a Rhenium Pincer System, Inorg. Chem. 2021, 60, 6115-6124.
Materna, K. L.; Jiang, J.; Crabtree, R. H.; Brudvig, G. W., Silatrane Anchors for Metal Oxide Surfaces: Optimization for Potential Photocatalytic and Electrocatalytic Applications, ACS Appl. Mater. Interfaces. 2018, 11, 5602-5609. DOI: 10.1021/acsami.8b04138
Rudshteyn, B.; Fisher, K. J.; Lant, H. M. C.; Yang, K. R.; Mercado, B.Q.; Brudvig, G.W.; Crabtree, R.H.; Batista, V.S., Water-Nucleophilic Attack Mechanism for the CuII(pyalk)2 Water-Oxidation Catalyst, ACS Catal. 2018, 8, 7952-7960.
Peris, E.; Crabtree, R. H. Key factors in pincer ligand design, Chem. Soc. Rev. 2018, 47, 1959-1968.
Sharninghausen, L. S.; Sinha, S. B.; Shopov, D. Y.; Balcells, D.; Brudvig, G. W.; Crabtree, R. H., Synthesis and Characterization of Iridium(V) Coordination Complexes With an N,O-Donor Organic Ligand. Angew. Chem. Int. Ed. 2017, 56, 12047-51.
Michaelos, T.; Shopov, D. Y.; Sinha, S. B.; Sharninghausen, L. S.; Fisher, K.; Lant, H.; Crabtree, R. H.; Brudvig, G. W. A Pyridine Alkoxide Chelate Ligand that Promotes Both Unusually High Oxidation States and Water-Oxidation Catalysis, Acc. Chem. Res. 2017, 50, 952-959.